Exciton Dynamics in Lead Halide Perovskite Nanocrystals

Exciton Dynamics in Lead Halide Perovskite Nanocrystals PDF Author: Bernhard Johann Bohn
Publisher:
ISBN: 9783030709419
Category :
Languages : en
Pages : 0

Get Book

Book Description
Less than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission. In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as the active layer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before.

Exciton Dynamics in Lead Halide Perovskite Nanocrystals

Exciton Dynamics in Lead Halide Perovskite Nanocrystals PDF Author: Bernhard Johann Bohn
Publisher:
ISBN: 9783030709419
Category :
Languages : en
Pages : 0

Get Book

Book Description
Less than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission. In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as the active layer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before.

Exciton Dynamics in Lead Halide Perovskite Nanocrystals

Exciton Dynamics in Lead Halide Perovskite Nanocrystals PDF Author: Bernhard Johann Bohn
Publisher: Springer Nature
ISBN: 303070940X
Category : Science
Languages : en
Pages : 169

Get Book

Book Description
Less than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission. In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as the active layer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before.

Halide Perovskites

Halide Perovskites PDF Author: Tze-Chien Sum
Publisher: John Wiley & Sons
ISBN: 3527341110
Category : Technology & Engineering
Languages : en
Pages : 312

Get Book

Book Description
Real insight from leading experts in the field into the causes of the unique photovoltaic performance of perovskite solar cells, describing the fundamentals of perovskite materials and device architectures. The authors cover materials research and development, device fabrication and engineering methodologies, as well as current knowledge extending beyond perovskite photovoltaics, such as the novel spin physics and multiferroic properties of this family of materials. Aimed at a better and clearer understanding of the latest developments in the hybrid perovskite field, this is a must-have for material scientists, chemists, physicists and engineers entering or already working in this booming field.

Halide Perovskite Semiconductors

Halide Perovskite Semiconductors PDF Author: Yuanyuan Zhou
Publisher: John Wiley & Sons
ISBN: 3527829032
Category : Science
Languages : en
Pages : 517

Get Book

Book Description
Halide Perovskite Semiconductors Enables readers to acquire a systematic and in-depth understanding of various fundamental aspects of halide perovskite semiconductors Halide Perovskite Semiconductors: Structures, Characterization, Properties, and Phenomena covers the most fundamental topics with regards to halide perovskites, including but not limited to crystal/defect theory, crystal chemistry, heterogeneity, grain boundaries, single-crystals/thin-films/nanocrystals synthesis, photophysics, solid-state ionics, spin physics, chemical (in)stability, carrier dynamics, hot carriers, surface and interfaces, lower-dimensional structures, and structural/functional characterizations. Included discussions on the fundamentals of halide perovskites aim to expand the basic science fields of physics, chemistry, and materials science. Edited by two highly qualified researchers, Halide Perovskite Semiconductors includes specific information on: Crystal/defect theory of halide perovskites, crystal chemistry of halide perovskites, and processing and microstructures of halide perovskites Single-crystals of halide perovskites, nanocrystals of halide perovskites, low-dimensional perovskite crystals, and nanoscale heterogeneity of halide perovskites Carrier mobilities and dynamics in halide perovskites, light emission of halide perovskites, photophysics and ultrafast spectroscopy of halide perovskites Hot carriers in halide perovskites, correlating photophysics with microstructures in halide perovskites, chemical stability of halide perovskites, and solid-state ionics of halide perovskites Readers can find solutions to technological issues and challenges based on the fundamental knowledge gained from this book. As such, Halide Perovskite Semiconductors is an essential in-depth treatment of the subject, ideal for solid-state chemists, materials scientists, physical chemists, inorganic chemists, physicists, and semiconductor physicists.

Semiconductor Nanocrystals

Semiconductor Nanocrystals PDF Author: Alexander L. Efros
Publisher: Springer Science & Business Media
ISBN: 1475736770
Category : Technology & Engineering
Languages : en
Pages : 277

Get Book

Book Description
A physics book that covers the optical properties of quantum-confined semiconductor nanostructures from both the theoretical and experimental points of view together with technological applications. Topics to be reviewed include quantum confinement effects in semiconductors, optical adsorption and emission properties of group IV, III-V, II-VI semiconductors, deep-etched and self assembled quantum dots, nanoclusters, and laser applications in optoelectronics.

Optical Properties of Low-dimensional Materials

Optical Properties of Low-dimensional Materials PDF Author: Tetsuo Ogawa
Publisher: World Scientific
ISBN: 9789810230487
Category : Science
Languages : en
Pages : 478

Get Book

Book Description
This book surveys recent theoretical and experimental studies of optical properties of low-dimensional materials. As an extended version of Optical Properties of Low-Dimensional Materials (Volume 1, published in 1995 by World Scientific), Volume 2 covers a wide range of interesting low-dimensional materials including both inorganic and organic systems, such as disordered polymers, deformable molecular crystals, dilute magnetic semiconductors, SiGe/Si short-period superlattices, GaAs quantum wires, semiconductor microcavities, and photonic crystals. There are excellent review articles by promising researchers in each field. All the materials introduced in this book yield new optical phenomena originating from their mesoscopic and low-dimensional electronic characters and electron-lattice couplings, which offer a new research field of materials science as well as condensed-matter and optical physics. Volumes 1 and 2 are interrelated but can be read independently. They are pitched at the level of graduate students and are useful to both students and scientists.

Quantum-dot Based Light-emitting Diodes

Quantum-dot Based Light-emitting Diodes PDF Author: Morteza Sasani Ghamsari
Publisher: BoD – Books on Demand
ISBN: 9535135759
Category : Technology & Engineering
Languages : en
Pages : 171

Get Book

Book Description
Quantum dot-based light emitting diodes were assigned to bringing together the latest and most important progresses in light emitting diode (LED) technologies. In addition, they were dedicated to gain the perspective of LED technology for all of its advancements and innovations due to the employment of semiconductor nanocrystals. Highly selective, the primary aim was to provide a visual source for high-urgency work that will define the future directions relating to the organic light emitting diode (OLED), with the expectation for lasting scientific and technological impact. The editor hopes that the chapters verify the realization of the mentioned aims that have been considered for editing of this book. Due to the rapidly growing OLED technology, we wish this book to be useful for any progress that can be achieved in future.

Nanoscale Materials

Nanoscale Materials PDF Author: Luis M. Liz-Marzán
Publisher: Springer Science & Business Media
ISBN: 0306481081
Category : Science
Languages : en
Pages : 500

Get Book

Book Description
Organized nanoassemblies of inorganic nanoparticles and organic molecules are building blocks of nanodevices, whether they are designed to perform molecular level computing, sense the environment or improve the catalytic properties of a material. The key to creation of these hybrid nanostructures lies in understanding the chemistry at a fundamental level. This book serves as a reference book for researchers by providing fundamental understanding of many nanoscopic materials.

Excitonic Processes in Solids

Excitonic Processes in Solids PDF Author: Masayasu Ueta
Publisher: Springer Science & Business Media
ISBN: 3642826024
Category : Science
Languages : en
Pages : 544

Get Book

Book Description
An exciton is an electronic excitation wave consisting of an electron-hole pair which propagates in a nonmetallic solid. Since the pioneering research of Fren kel, Wannier and the Pohl group in the 1930s, a large number of experimental and theoretical studies have been made. Due to these investigations the exciton is now a well-established concept and the electronic structure has been clarified in great detail. The next subjects for investigation are, naturally, dynamical processes of excitons such as excitation, relaxation, annihilation and molecule formation and, in fact, many interesting phenomena have been disclosed by recent works. These excitonic processes have been recognized to be quite important in solid-state physics because they involve a number of basic interactions between excitons and other elementary excitations. It is the aim of this quasi monograph to describe these excitonic processes from both theoretical and experimental points of view. we take a few To discuss and illustrate the excitonic processes in solids, important and well-investigated insulating crystals as playgrounds for excitons on which they play in a manner characteristic of each material. The selection of the materials is made in such a way that they possess some unique properties of excitonic processes and are adequate to cover important interactions in which excitons are involved. In each material, excitonic processes are described in detail from the experimental side in order to show the whole story of excitons in a particular material.

Self-Trapped Excitons

Self-Trapped Excitons PDF Author: K.S. Song
Publisher: Springer Science & Business Media
ISBN: 364285236X
Category : Technology & Engineering
Languages : en
Pages : 426

Get Book

Book Description
Self-Trapped Excitons discusses the structure and evolution of the self-trapped exciton (STE) in a wide range of materials. It includes a comprehensive review of experiments and extensive tables of data. Emphasis is given throughout to the unity of the basic physics underlying various manifestations of self-trapping, with the theory being developed from a localized, atomistic perspective. The topics treated in detail in relation to STE relaxation include spontaneous symmetry breaking, lattice defect formation, radiation damage, and electronic sputtering.