Ultrafast Dynamics of Coulomb Correlated Excitons in GaAs Quantum Wells PDF Download
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Author: Mary-Ann Mycek
Publisher:
ISBN:
Category :
Languages : en
Pages : 368
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Book Description
Author: Mary-Ann Mycek
Publisher:
ISBN:
Category :
Languages : en
Pages : 368
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Book Description
Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 182
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Book Description
The author measures the transient nonlinear optical response of room temperature excitons in gallium arsenide quantum wells via multi-wave mixing experiments. The dynamics of the resonantly excited excitons is directly reflected by the ultrafast decay of the induced nonlinear polarization, which radiates the detected multi-wave mixing signal. She characterizes this ultrafast coherent emission in both amplitude and phase, using time- and frequency-domain measurement techniques, to better understand the role of Coulomb correlation in these systems. To interpret the experimental results, the nonlinear optical response of a dense medium is calculated using a model including Coulomb interaction. She contributes three new elements to previous theoretical and experimental studies of these systems. First, surpassing traditional time-integrated measurements, she temporally resolves the amplitude of the ultrafast coherent emission. Second, in addition to measuring the third-order four-wave mixing signal, she also investigates the fifth-order six-wave mixing response. Third, she characterizes the ultrafast phase dynamics of the nonlinear emission using interferometric techniques with an unprecedented resolution of approximately 140 attoseconds. The author finds that effects arising from Coulomb correlation dominate the nonlinear optical response when the density of excitons falls below 3 x 1011 cm−2, the saturation density. These signatures of Coulomb correlation are investigated for increasing excitation density to gradually screen the interactions and test the validity of the model for dense media. The results are found to be qualitatively consistent with both the predictions of the model and with numerical solutions to the semiconductor Bloch equations. Importantly, the results also indicate current experimental and theoretical limitations, which should be addressed in future research.
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Languages : en
Pages :
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Author:
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Category :
Languages : en
Pages : 26
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Author: Neil Primozich
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Category : Coulomb functions
Languages : en
Pages : 256
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Author: J. B. Stark
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Category :
Languages : en
Pages : 4
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Spatial confinement along one dimension, using the methods of epitaxial crystal growth, has demonstrated that linear and nonlinear optical properties depend strongly on dimensionality. Confinement along the remaining directions, however, continues to present formidable technological obstacles. Difficulties in the control of the surface properties and size distribution of quantum dots and semiconductor microcrystallites results in materials with unsatisfactory optical quality. Confinement along all three dimensions can be achieved, in materials of excellent optical quality, by placing a quantum well material in a perpendicular magnetic field. As the field is increased, the extension of the resulting electronic orbitals decreases, so that the dimensionality of the states may be tuned from two to zero dimensions. Using femtosecond excite-and-probe optical techniques in fields as large as 12 Tesla, we measure the time resolved dynamics of zero dimensional magneto-excitons.
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Category : Aeronautics
Languages : en
Pages : 692
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Category : Power resources
Languages : en
Pages : 508
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Category : Dissertation abstracts
Languages : en
Pages : 872
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Publisher: Elsevier
ISBN: 0080541003
Category : Science
Languages : en
Pages : 514
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Book Description
Since its inception in 1966, the series of numbered volumes known as Semiconductors and Semimetals has distinguished itself through the careful selection of well-known authors, editors, and contributors. The Willardson and Beer series, as it is widely known, has succeeded in producing numerous landmark volumes and chapters. Not only did many of these volumes make an impact at the time of their publication, but they continue to be well-cited years after their original release. Recently, Professor Eicke R. Weber of the University of California at Berkeley joined as a co-editor of the series. Professor Weber, a well-known expert in the field of semiconductor materials, will further contribute to continuing the series' tradition of publishing timely, highly relevant, and long-impacting volumes. Some of the recent volumes, such as Hydrogen in Semiconductors, Imperfections in III/V Materials, Epitaxial Microstructures, High-Speed Heterostructure Devices, Oxygen in Silicon, and others promise that this tradition will be maintained and even expanded.
