Local Investigation of Single Magnetic Molecules with Scanning Tunneling Microscopy

Local Investigation of Single Magnetic Molecules with Scanning Tunneling Microscopy PDF Author: Chen, Jinjie
Publisher: KIT Scientific Publishing
ISBN: 3731508192
Category : Molecules
Languages : en
Pages : 146

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Book Description
We worked on different magnetic molecules containing 3d and 4f magnetic centers. Their growth on metallic surfaces, topographies, spin states, magnetic properties and electron transport were locally investigated by using scanning tunneling microscopy (STM) at temperatures down to 30mK. The main achievement of this dissertation reveals the abrupt switching of crystal fields during formation of molecular contacts.

Local Investigation of Single Magnetic Molecules with Scanning Tunneling Microscopy

Local Investigation of Single Magnetic Molecules with Scanning Tunneling Microscopy PDF Author: Chen, Jinjie
Publisher: KIT Scientific Publishing
ISBN: 3731508192
Category : Molecules
Languages : en
Pages : 146

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Book Description
We worked on different magnetic molecules containing 3d and 4f magnetic centers. Their growth on metallic surfaces, topographies, spin states, magnetic properties and electron transport were locally investigated by using scanning tunneling microscopy (STM) at temperatures down to 30mK. The main achievement of this dissertation reveals the abrupt switching of crystal fields during formation of molecular contacts.

Local Investigation of Single Magnetic Molecules With Scanning Tunneling Microscopy

Local Investigation of Single Magnetic Molecules With Scanning Tunneling Microscopy PDF Author: Jinjie Chen
Publisher:
ISBN: 9781013278945
Category : Science
Languages : en
Pages : 138

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Book Description
We worked on different magnetic molecules containing 3d and 4f magnetic centers. Their growth on metallic surfaces, topographies, spin states, magnetic properties and electron transport were locally investigated by using scanning tunneling microscopy (STM) at temperatures down to 30mK. The main achievement of this dissertation reveals the abrupt switching of crystal fields during formation of molecular contacts. This work was published by Saint Philip Street Press pursuant to a Creative Commons license permitting commercial use. All rights not granted by the work's license are retained by the author or authors.

Local Probing of a Superconductor’s Quasiparticles and Bosonic Excitations with a Scanning Tunnelling Microscope

Local Probing of a Superconductor’s Quasiparticles and Bosonic Excitations with a Scanning Tunnelling Microscope PDF Author: Gozlinski, Thomas
Publisher: KIT Scientific Publishing
ISBN: 3731512793
Category : Science
Languages : en
Pages : 208

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Book Description
Complementary to scattering techniques, scanning tunnelling microscopy provides atomic-scale real space information about a material's electronic state of matter. State-of-the-art designs of a scanning tunnelling microscope (STM) allow measurements at millikelvin temperatures with unprecedented energy resolution. Therefore, this instrument excels in probing the superconducting state at low temperatures and especially its local quasiparticle excitations as well as bosonic degrees of freedom.

Light Emission from Single Self-decoupled Molecules in a Scanning Tunnelling Microscope

Light Emission from Single Self-decoupled Molecules in a Scanning Tunnelling Microscope PDF Author: Rai, Vibhuti Narayan
Publisher: KIT Scientific Publishing
ISBN: 3731512017
Category : Science
Languages : en
Pages : 150

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Book Description
In this work, a clear pathway is presented to achieve well-defined electronically decoupled chromophores from metallic leads without requiring additional insulating layers. To study such self-decoupled molecules, STM equipped with an efficient light detection setup has been used. Results show that the chromophores mounted on tripodal molecular platforms adsorbed on a gold surface present well-defined and efficient electroluminescence down to the single-molecule level.

Molecular Motor Based on Single Chiral Tripodal Molecules Studied with STM

Molecular Motor Based on Single Chiral Tripodal Molecules Studied with STM PDF Author: Skolaut, Julian
Publisher: KIT Scientific Publishing
ISBN: 3731512475
Category :
Languages : en
Pages : 164

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Book Description
This work presents a single molecular motor driven by the current in an STM. Its chiral functional group is supposed to perform a rotation in a preferred direction, proven by Binomial tests to be statistically significant. The rotation is proposedly driven by the chiral-induced spin selectivity effect (CISS). However, the studies of the rotation on the dependence on the lateral tip position, voltage and current indicate that he CISS is unlikely to cause the preferred rotation direction.

Adding nonlinearity to an electromagnetic-magnonic quantum hybrid device

Adding nonlinearity to an electromagnetic-magnonic quantum hybrid device PDF Author: Pfirrmann, Marco
Publisher: KIT Scientific Publishing
ISBN: 3731510030
Category : Science
Languages : en
Pages : 136

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Book Description
In this book, hybrid systems based on yttrium-iron-garnet (YIG), three dimensional microwave cavity resonators, and superconducting transmon qubits, are investigated by continuous wave and pulsed microwave spectroscopy. Limitations to the magnetic linewidth in the quantum regime are identified and coherent exchange between a magnon and a superconducting qubit are demonstrated. Finally, a first step towards a strongly coupled hybrid system containing all three components is demonstrated.

Quantum Sensing Experiments with Superconducting Qubits

Quantum Sensing Experiments with Superconducting Qubits PDF Author: Schneider, Andre
Publisher: KIT Scientific Publishing
ISBN: 3731510324
Category : Science
Languages : en
Pages : 170

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Book Description
Quantum sensing is a vast and emerging field enabling in-situ studies of quantum systems and hence the development of quantum hybrid systems. This work creates the fundament of direct superconducting-magnetic hybrid systems by developing a local microwave sensing scheme and studying the influence of a static magnetic field on a superconducting qubit. Finally, a proof-of-principle hybrid system is demonstrated, which opens the path towards superconducting-magnetic quantum circuits.

Sub-Kelvin scanning tunneling microscopy on magnetic molecules

Sub-Kelvin scanning tunneling microscopy on magnetic molecules PDF Author: Zhang, Lei
Publisher: KIT Scientific Publishing
ISBN: 386644950X
Category : Science
Languages : en
Pages : 116

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Book Description


Scanning Tunneling Spectroscopy of Magnetic Bulk Impurities

Scanning Tunneling Spectroscopy of Magnetic Bulk Impurities PDF Author: Henning Prüser
Publisher: Springer
ISBN: 3319063855
Category : Science
Languages : en
Pages : 117

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Book Description
Magnetic impurities in a non-magnetic host metal have been actively explored in condensed matter physics in recent last decades. From both fundamental and applied viewpoints these systems are very interesting because they can exhibit strong electronic correlations that give rise to various fascinating phenomena beyond the single particle picture. Up to now our understanding of the underlying processes remains limited due to difficulties involved in measuring these systems on a microscopic scale. With their unique control, scanning tunneling microscopy (STM) and spectroscopy (STS) allow for the first time investigations of phenomena occurring on very small length and energy scales. Here, single magnetic iron and cobalt atoms embedded beneath a metal surface are investigated using these techniques. In particular, the transition from single impurity Kondo physics to two interacting impurities is studied in real space. This thesis contains a comprehensive description of the STM /STS technique, sub-surface impurities, as well as single- and two-impurity Kondo physics - and as such offers a valuable introduction to newcomers to the field.

Elastic and Inelastic Scanning Tunneling Spectroscopy on Iron-Based Superconductors

Elastic and Inelastic Scanning Tunneling Spectroscopy on Iron-Based Superconductors PDF Author: Jandke, Jasmin Maria
Publisher: KIT Scientific Publishing
ISBN: 3731507471
Category : Physics
Languages : en
Pages : 242

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Book Description
Within this work, the pairing mechanism of conventional (Pb) and unconventional superconductors (SrFe2(As1-xPx )2 , FeSe, FeSe/STO) was investigated experimentally by means of elastic and inelastic tunneling spectroscopy at temperatures down to 30 mK. The distinction between elastic and inelastic contributions to tunneling data was elaborated. The results help to identify conventional (phonon-mediated) and unconventional (e.g. spin-?uctuation mediated) superconductivity.