Amorphization kinetics of Zr3Fe under electron irradiation

Amorphization kinetics of Zr3Fe under electron irradiation PDF Author: Chalk River Nuclear Laboratories. Reactor Materials Research Branch
Publisher: Chalk River, Ont. : Reactor Materials Research Branch, Chalk River Laboratories
ISBN: 9780660159003
Category : Irradiation
Languages : en
Pages : 16

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Amorphization Kinetics of Zr3Fe Under Electron Irradiation

Amorphization Kinetics of Zr3Fe Under Electron Irradiation PDF Author:
Publisher:
ISBN:
Category :
Languages : en
Pages :

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Amorphization Kinetics of Zr{sub 3}Fe Under Electron Irradiation

Amorphization Kinetics of Zr{sub 3}Fe Under Electron Irradiation PDF Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 16

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0.9 MeV electron irradiations were performed at 28--220 K in a high-voltage electron microscope (HVEM). By measuring onset, spread and final size of the amorphous region, factoring in the Guassian distribution of the beam, a kinetic description of the amorphization in terms of dose, dose rate and temperature was obtained. The critical temperature for amorphization by electron irradiation was found to be ∼220 K, compared to 570--625 K for 4°Ar ion irradiation. Also, the dose-to-amorphization increased exponentially with temperature. Results indicated that the rate of growth of the amorphous region under the electron beam decreased with increasing temperature and the does-to-amorphization decreased with increasing dose rate. The size of the amorphous region saturated after a region dose, the final size decreasing with increasing temperature, and it was argued that this is related to the existence of a critical dose rate, which increased with temperature, below which no amorphization occurred. The above observations can be understood in the framework of the kinetics of damage accumulation under irradiation.

Energy Research Abstracts

Energy Research Abstracts PDF Author:
Publisher:
ISBN:
Category : Power resources
Languages : en
Pages : 806

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Semiannual, with semiannual and annual indexes. References to all scientific and technical literature coming from DOE, its laboratories, energy centers, and contractors. Includes all works deriving from DOE, other related government-sponsored information, and foreign nonnuclear information. Arranged under 39 categories, e.g., Biomedical sciences, basic studies; Biomedical sciences, applied studies; Health and safety; and Fusion energy. Entry gives bibliographical information and abstract. Corporate, author, subject, report number indexes.

Electron Energy Dependence of Amorphization in Zr3Fe

Electron Energy Dependence of Amorphization in Zr3Fe PDF Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 7

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This paper reports the results from a study conducted to determine the effect of electron energy on the dose-to-amorphization of Zr{sub 3,}Fe at 23--30 K. Zr3Fe samples were irradiated in the HVEM at Argonne National Laboratory, at 200 to 900 keV. Amorphization occurred at electron energies from 900 keV down to 250 keV. Three distinct regions were observed: between 900 and 700 key amorphization occurred at a constant low dose of (approximately) 4 x 1021 e cm−2; a higher plateau at 1022 was observed between 600 and 400 keV, and finally there was a sharp increase in the dose-to-amorphization below 400 key, so that at 250 key the necessary dose was an order of magnitude higher than that at 900 keV. In the region below 400 keV there was evidence of a dependence of the dose-to-amorphization on the orientation of the sample with respect to the electron beam. The results can be analyzed in terms of a composite displacement cross section dominated at high energies by displacements of Zr and Fe atoms, by displacements of Fe atoms at intermediate energies and of secondary displacements of lattice atoms by recoil impurities at low energies.

Amorphization Kinetics of Zr(Cr, Fe)2 Under Ion Irradiation

Amorphization Kinetics of Zr(Cr, Fe)2 Under Ion Irradiation PDF Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 7

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Thin foils of Zircaloy-4 were irradiated with 350 KeV 4°Ar ions in the dual ion beam/HVEM facility at Argonne National Laboratory at 300--650 K. The irradiation-induced amorphization of the intermetallic precipitates Zr (Cr; Fe)2 and Zr2 (Ni, Fe) was studied in-situ. For Zr (Cr, Fe)2 precipitates the dose-to-amorphization was found to increase exponentially with temperature, with a critical temperature of about 650 K. The amorphization morphology was shown to be homogeneous, with no preferential site for nucleation, in contrast to neutron-irradiation amorphization which started at the precipitate-matrix interface. For Zr2 (Ni, Fe) precipitates it was found that amorphization occurred at 550 and 600 K, whereas in neutron irradiation no amorphization has been observed at those temperatures. The results are discussed in context of previous neutron and electron irradiations and likely amorphization mechanisms are proposed.

Amorphization Kinetics of Zr(Cr, Fe)[sub 2] Under Ion Irradiation

Amorphization Kinetics of Zr(Cr, Fe)[sub 2] Under Ion Irradiation PDF Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 7

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Thin foils of Zircaloy-4 were irradiated with 350 KeV [sup 40]Ar ions in the dual ion beam/HVEM facility at Argonne National Laboratory at 300--650 K. The irradiation-induced amorphization of the intermetallic precipitates Zr (Cr; Fe)[sub 2] and Zr[sub 2] (Ni, Fe) was studied in-situ. For Zr (Cr, Fe)[sub 2] precipitates the dose-to-amorphization was found to increase exponentially with temperature, with a critical temperature of about 650 K. The amorphization morphology was shown to be homogeneous, with no preferential site for nucleation, in contrast to neutron-irradiation amorphization which started at the precipitate-matrix interface. For Zr[sub 2] (Ni, Fe) precipitates it was found that amorphization occurred at 550 and 600 K, whereas in neutron irradiation no amorphization has been observed at those temperatures. The results are discussed in context of previous neutron and electron irradiations and likely amorphization mechanisms are proposed.

Microstructure of Irradiated Materials: Volume 373

Microstructure of Irradiated Materials: Volume 373 PDF Author: Ian M. Robertson
Publisher:
ISBN:
Category : Science
Languages : en
Pages : 600

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Book Description
The focus of the symposium, which was held at the 1994 MRS Fall Meeting, was on the changes produced in the microstructure of metals, ceramics, and semiconductors by irradiation with energetic particles. This proceedings volume contains invited and contributed papers. Among the topics are computer simulation of displacement cascade damage in metals; radiation effects in ceramic insulators; and computer simulation of thermal annealing effects of self implanted silicon. Annotation copyright by Book News, Inc., Portland, OR

Amorphization Kinetics of Zr(Cr, Fe)2 Under Ion Irradiation

Amorphization Kinetics of Zr(Cr, Fe)2 Under Ion Irradiation PDF Author: Arthur T. Motta
Publisher: Chalk River, Ont. : Reactor Materials Research Branch
ISBN: 9780660158969
Category : Amorphous substances
Languages : en
Pages : 9

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Comprehensive Nuclear Materials

Comprehensive Nuclear Materials PDF Author:
Publisher: Elsevier
ISBN: 0081028660
Category : Science
Languages : en
Pages : 4871

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Book Description
Materials in a nuclear environment are exposed to extreme conditions of radiation, temperature and/or corrosion, and in many cases the combination of these makes the material behavior very different from conventional materials. This is evident for the four major technological challenges the nuclear technology domain is facing currently: (i) long-term operation of existing Generation II nuclear power plants, (ii) the design of the next generation reactors (Generation IV), (iii) the construction of the ITER fusion reactor in Cadarache (France), (iv) and the intermediate and final disposal of nuclear waste. In order to address these challenges, engineers and designers need to know the properties of a wide variety of materials under these conditions and to understand the underlying processes affecting changes in their behavior, in order to assess their performance and to determine the limits of operation. Comprehensive Nuclear Materials, Second Edition, Seven Volume Set provides broad ranging, validated summaries of all the major topics in the field of nuclear material research for fission as well as fusion reactor systems. Attention is given to the fundamental scientific aspects of nuclear materials: fuel and structural materials for fission reactors, waste materials, and materials for fusion reactors. The articles are written at a level that allows undergraduate students to understand the material, while providing active researchers with a ready reference resource of information. Most of the chapters from the first Edition have been revised and updated and a significant number of new topics are covered in completely new material. During the ten years between the two editions, the challenge for applications of nuclear materials has been significantly impacted by world events, public awareness, and technological innovation. Materials play a key role as enablers of new technologies, and we trust that this new edition of Comprehensive Nuclear Materials has captured the key recent developments. Critically reviews the major classes and functions of materials, supporting the selection, assessment, validation and engineering of materials in extreme nuclear environments Comprehensive resource for up-to-date and authoritative information which is not always available elsewhere, even in journals Provides an in-depth treatment of materials modeling and simulation, with a specific focus on nuclear issues Serves as an excellent entry point for students and researchers new to the field