The Impact of Meteorological Conditions and Variation in Chemical Composition of Aerosols on Regional Cloud Formation

The Impact of Meteorological Conditions and Variation in Chemical Composition of Aerosols on Regional Cloud Formation PDF Author: Jessie Marie Creamean
Publisher:
ISBN: 9781267646668
Category :
Languages : en
Pages : 236

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Book Description
Atmospheric aerosols have significant implications for human health and climate. For instance, aerosols impact climate directly by scattering and absorbing solar and terrestrial radiation and indirectly by acting as cloud condensation nuclei (CCN) and ice nuclei (IN), which facilitate cloud droplet and ice crystal formation, respectively. Changes in chemistry, size, and number concentrations between different locations and over time alter how aerosols impact air quality and cloud formation, and can have broader implications on precipitation efficiency and phase. Further, aerosol composition largely depends on meteorology, which influences sources and chemical transformation in the atmosphere. Aerosol-cloud-precipitation interactions represent one of the largest sources of uncertainty in climate science; therefore, a better understanding of the aerosols that contribute to these effects is needed. To address this source of uncertainty, the chemical composition of individual ambient aerosols and aerosols as insoluble residues in precipitation samples was determined using aerosol time-of-flight mass spectrometry (ATOFMS) and provided insight into their potential to serve as cloud seeds at three different locations over time. A three-year summer study (2005-2007) in Riverside, CA afforded information on the inter-annual variability of the urban aerosol due to changes in aerosol transport and meteorological conditions. In the summer of 2008 in Atlanta, GA, tropical cyclones shifted the representative aged urban aerosol to a less-aged, less-CCN active aerosol population, having implications on regional cloud formation after extreme weather events. At a remote site in the Sierra Nevada Mountains in the winter of 2009, observations of newly-formed aerosols presented a new source of CCN. Inter-annual trends in precipitation at the same remote site showed how IN transported from the Sahara and Asia potentially influenced precipitation processes during three winter seasons (2009-2011). Investigating changes in cloud seeds represents a longer-term goal to reduce uncertainties associated with modeling aerosol-cloud-precipitation interactions. Larger spatial and temporal coverage is needed to better understand trends in cloud formation and precipitation and to provide more detail for regional and global model parameterization. The results presented herein represent a noteworthy advancement towards understanding variation in composition and sources of cloud seeds in different regions and in most cases long time periods.

The Impact of Meteorological Conditions and Variation in Chemical Composition of Aerosols on Regional Cloud Formation

The Impact of Meteorological Conditions and Variation in Chemical Composition of Aerosols on Regional Cloud Formation PDF Author: Jessie Marie Creamean
Publisher:
ISBN: 9781267646668
Category :
Languages : en
Pages : 236

Get Book Here

Book Description
Atmospheric aerosols have significant implications for human health and climate. For instance, aerosols impact climate directly by scattering and absorbing solar and terrestrial radiation and indirectly by acting as cloud condensation nuclei (CCN) and ice nuclei (IN), which facilitate cloud droplet and ice crystal formation, respectively. Changes in chemistry, size, and number concentrations between different locations and over time alter how aerosols impact air quality and cloud formation, and can have broader implications on precipitation efficiency and phase. Further, aerosol composition largely depends on meteorology, which influences sources and chemical transformation in the atmosphere. Aerosol-cloud-precipitation interactions represent one of the largest sources of uncertainty in climate science; therefore, a better understanding of the aerosols that contribute to these effects is needed. To address this source of uncertainty, the chemical composition of individual ambient aerosols and aerosols as insoluble residues in precipitation samples was determined using aerosol time-of-flight mass spectrometry (ATOFMS) and provided insight into their potential to serve as cloud seeds at three different locations over time. A three-year summer study (2005-2007) in Riverside, CA afforded information on the inter-annual variability of the urban aerosol due to changes in aerosol transport and meteorological conditions. In the summer of 2008 in Atlanta, GA, tropical cyclones shifted the representative aged urban aerosol to a less-aged, less-CCN active aerosol population, having implications on regional cloud formation after extreme weather events. At a remote site in the Sierra Nevada Mountains in the winter of 2009, observations of newly-formed aerosols presented a new source of CCN. Inter-annual trends in precipitation at the same remote site showed how IN transported from the Sahara and Asia potentially influenced precipitation processes during three winter seasons (2009-2011). Investigating changes in cloud seeds represents a longer-term goal to reduce uncertainties associated with modeling aerosol-cloud-precipitation interactions. Larger spatial and temporal coverage is needed to better understand trends in cloud formation and precipitation and to provide more detail for regional and global model parameterization. The results presented herein represent a noteworthy advancement towards understanding variation in composition and sources of cloud seeds in different regions and in most cases long time periods.

Atmospheric Aerosols

Atmospheric Aerosols PDF Author: Hayder Abdul-Razzak
Publisher: BoD – Books on Demand
ISBN: 9535107283
Category : Science
Languages : en
Pages : 494

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Book Description
The book is divided into two sections. The first section presents characterization of atmospheric aerosols and their impact on regional climate from East Asia to the Pacific. Ground-based, air-born, and satellite data were collected and analyzed. Detailed information about measurement techniques and atmospheric conditions were provided as well. In the second section, authors provide detailed information about the organic and inorganic constituents of atmospheric aerosols. They discuss the chemical and physical processes, temporal and spatial distribution, emissions, formation, and transportation of aerosol particles. In addition, new measurement techniques are introduced. This book hopes to serve as a useful resource to resolve some of the issues associated with the complex nature of the interaction between atmospheric aerosols and climatology.

Atmospheric Aerosol Properties

Atmospheric Aerosol Properties PDF Author: Kirill Ya. Kondratyev
Publisher: Springer Science & Business Media
ISBN: 3540376984
Category : Science
Languages : en
Pages : 595

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Book Description
This book provides the first comprehensive analysis of how aerosols form in the atmosphere through in situ processes as well as via transport from the surface (dust storms, seas spray, biogenic emissions, forest fires etc.). Such an analysis has been followed by the consideration of both observation data (various field observational experiments) and numerical modeling results to assess climate impacts of aerosols bearing in mind that these impacts are the most significant uncertainty in studying natural and anthropogenic causes of climate change.

Atmospheric Aerosol Properties

Atmospheric Aerosol Properties PDF Author: Kirill Ya. Kondratyev
Publisher: Springer
ISBN: 9783540262633
Category : Science
Languages : en
Pages : 572

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Book Description
This book provides the first comprehensive analysis of how aerosols form in the atmosphere through in situ processes as well as via transport from the surface (dust storms, seas spray, biogenic emissions, forest fires etc.). Such an analysis has been followed by the consideration of both observation data (various field observational experiments) and numerical modeling results to assess climate impacts of aerosols bearing in mind that these impacts are the most significant uncertainty in studying natural and anthropogenic causes of climate change.

Atmospheric Aerosol Properties and Climate Impacts

Atmospheric Aerosol Properties and Climate Impacts PDF Author:
Publisher:
ISBN:
Category : Atmospheric ozone
Languages : en
Pages : 128

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Book Description


Quantifying Compositional Impacts of Ambient Aerosol on Cloud Formation

Quantifying Compositional Impacts of Ambient Aerosol on Cloud Formation PDF Author: Sara Lance
Publisher:
ISBN:
Category : Aerosols
Languages : en
Pages :

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Book Description
It has been historically assumed that most of the uncertainty associated with the aerosol indirect effect on climate can be attributed to the unpredictability of updrafts. We assess the sensitivity of cloud droplet number density to realistic variations in aerosol chemical properties and to variable updraft velocities using a 1-dimensional cloud parcel model. The results suggest that aerosol chemical variability may be as important to the aerosol indirect effect as the effect of unresolved cloud dynamics, especially in polluted environments. We next used a continuous flow streamwise thermal gradient Cloud Condesnation Nuclei counter (CCNc) to study the water-uptake properties of the ambient aerosol, by exposing an aerosol sample to a controlled water vapor supersaturation and counting the resulting number of droplets. The heat transfer properties and droplet growth within the CCNc were first modeled and experimentally characterized. We describe results from the MIRAGE field campaign at a ground-based site during March, 2006. Size-resolved CCN activation spectra and hygroscopic growth factor distributions of the ambient aerosol in Mexico City were obtained, and an analytical technique was developed to quantify a probability distribution of solute volume fractions for the CCN, as well as the aerosol mixing-state. The CCN were shown to be much less CCN active than ammonium sulfate, with water uptake properties more consistent with low molecular weight organic compounds. We also describe results from the GoMACCS field study, an airborne field campaign in Houston, Texas during August-September, 2006. GoMACCS tested our ability to predict CCN for highly polluted conditions with limited chemical information. Assuming the particles were composed purely of ammonium sulfate, CCN closure was obtained with a 10% overprediction bias on average for CCN concentrations ranging from less than 100 cm-3 to over 10,000 cm-3, but with on average 50% variability. Assuming measured concentrations of organics to be internally mixed and insoluble tended to reduce the overprediction bias for less polluted conditions, but led to underprediction bias in the most polluted conditions. Comparing the two campaigns, it is clear that the chemistry of the particles plays an important role in our ability to predict CCN concentrations.

Aerosols

Aerosols PDF Author: Konstantin Volkov
Publisher: BoD – Books on Demand
ISBN: 9535128434
Category : Technology & Engineering
Languages : en
Pages : 208

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Book Description
Aerosols have a significant impact on technological processes and human activities. In many cases, aerosols are at the core of human health, environmental and technological problems (climate change and air quality). However, aerosols can be successfully used in industry and technology (new materials, fire suppression and fuel delivery). The current scientific status of aerosol modelling and simulation and measurements and some advances in computational techniques, particle measurement technologies and practical applications of aerosols are reviewed and considered in this book. This book also includes a number of case studies focused on analysis of optical thickness and air quality in various regions.

Global Atmospheric Change and its Impact on Regional Air Quality

Global Atmospheric Change and its Impact on Regional Air Quality PDF Author: Ian Barnes
Publisher: Springer Science & Business Media
ISBN: 9401000824
Category : Science
Languages : en
Pages : 354

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Book Description
The NATO ARW in Irkutsk was an excellent occasion for the coming together of Eastern and Western scientists who are involved in tropospheric science; the workshop has greatly contributed to the scientific and social understanding among the participants from the many different countries. Many new personal contacts were made which will help to strengthen future collaborations. In particular, the Lake Baikal area and the Limnological Institute offer splendid opportunities for environmental research which, in part, is already on going. For most participants it was the first time to see the impressive nature of the Lake Baikal region. Hopefully, there will be a chance for a follow-up event in Siberia where researchers from the East and West can again meet and engage in fruitful scientific dialogue. The book contains extended abstracts of the lectures and the poster presentations presented at the NATO ARW "Global Atmospheric Change and its Impact on Regional Air Quality" Irkutsk, Lake Baikal, Russian Federation, August 21-27, 2001. The ARW was composed of 22 oral presentations by key lecturers and 6 additional shorter oral presentations from participants. In a special poster session the 36 poster contributions were presented and discussed. Unfortunately not all contributors submitted extended abstracts, however, to compensate two contributions have been added from 2 participants who were originally invited but were unable to attend.

A Plan for a Research Program on Aerosol Radiative Forcing and Climate Change

A Plan for a Research Program on Aerosol Radiative Forcing and Climate Change PDF Author: Panel on Aerosol Radiative Forcing and Climate Change
Publisher: National Academies Press
ISBN: 0309588871
Category : Science
Languages : en
Pages : 180

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Book Description
This book recommends the initiation of an "integrated" research program to study the role of aerosols in the predicted global climate change. Current understanding suggest that, even now, aerosols, primarily from anthropogenic sources, may be reducing the rate of warming caused by greenhouse gas emissions. In addition to specific research recommendations, this book forcefully argues for two kinds of research program integration: integration of the individual laboratory, field, and theoretical research activities and an integrated management structure that involves all of the concerned federal agencies.

Atmospheric Aerosol Properties and Climate Impacts

Atmospheric Aerosol Properties and Climate Impacts PDF Author: Mian Chin
Publisher: DIANE Publishing
ISBN: 1437912613
Category : Science
Languages : en
Pages : 128

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Book Description
This Synthesis and Assessment Product (SAP) critically reviews current knowledge about global distributions and properties of atmospheric aerosols, as they relate to aerosol impacts on climate. It assesses possible next steps aimed at substantially reducing uncertainties in aerosol radiative forcing estimates. Current measurement techniques and modeling approaches are summarized, providing context. The objectives of this report are: (1) to promote a consensus about the knowledge base for climate change decision support; and (2) to provide a synthesis and integration of the current knowledge of the climate-relevant impacts of anthropogenic aerosols. Illustrations.