High-Resolution Experiments on Strong-Field Ionization of Atoms and Molecules

High-Resolution Experiments on Strong-Field Ionization of Atoms and Molecules PDF Author: Lutz Fechner
Publisher: Springer
ISBN: 3319320467
Category : Science
Languages : en
Pages : 158

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Book Description
In this thesis, the ionization of atoms and small molecules in strong laser fields is experimentally studied using a reaction microscope. The population of autoionizing doubly excited states in the laser fields is proven and a possible connection to the well-known dielectronic recombination processes is discussed. The fundamental process of tunnel ionization in strong laser fields is subject of investigation in a pump-probe experiment with ultrashort laser pulses. A coherent superposition of electronic states in singly charged argon ions is created within the first, and subsequently tunnel-ionized with the second pulse. This gives access to state-selective information about the tunneling process and allows to test common models. Moreover, the ionization of krypton and argon at different wavelengths is studied, from the multiphoton to the tunneling regime. The wavelength-dependent investigations are furthermore extended to molecular hydrogen. In addition to ionization, this system might undergo different dissociative processes. Channel-selective electron momentum distributions are presented and compared to each other.

High-Resolution Experiments on Strong-Field Ionization of Atoms and Molecules

High-Resolution Experiments on Strong-Field Ionization of Atoms and Molecules PDF Author: Lutz Fechner
Publisher: Springer
ISBN: 3319320467
Category : Science
Languages : en
Pages : 158

Get Book Here

Book Description
In this thesis, the ionization of atoms and small molecules in strong laser fields is experimentally studied using a reaction microscope. The population of autoionizing doubly excited states in the laser fields is proven and a possible connection to the well-known dielectronic recombination processes is discussed. The fundamental process of tunnel ionization in strong laser fields is subject of investigation in a pump-probe experiment with ultrashort laser pulses. A coherent superposition of electronic states in singly charged argon ions is created within the first, and subsequently tunnel-ionized with the second pulse. This gives access to state-selective information about the tunneling process and allows to test common models. Moreover, the ionization of krypton and argon at different wavelengths is studied, from the multiphoton to the tunneling regime. The wavelength-dependent investigations are furthermore extended to molecular hydrogen. In addition to ionization, this system might undergo different dissociative processes. Channel-selective electron momentum distributions are presented and compared to each other.

Controlling the Quantum World

Controlling the Quantum World PDF Author: National Research Council
Publisher: National Academies Press
ISBN: 0309102707
Category : Science
Languages : en
Pages : 245

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Book Description
As part of the Physics 2010 decadal survey project, the Department of Energy and the National Science Foundation requested that the National Research Council assess the opportunities, over roughly the next decade, in atomic, molecular, and optical (AMO) science and technology. In particular, the National Research Council was asked to cover the state of AMO science, emphasizing recent accomplishments and identifying new and compelling scientific questions. Controlling the Quantum World, discusses both the roles and challenges for AMO science in instrumentation; scientific research near absolute zero; development of extremely intense x-ray and laser sources; exploration and control of molecular processes; photonics at the nanoscale level; and development of quantum information technology. This book also offers an assessment of and recommendations about critical issues concerning maintaining U.S. leadership in AMO science and technology.

Molecular Beams in Physics and Chemistry

Molecular Beams in Physics and Chemistry PDF Author: Bretislav Friedrich
Publisher: Springer Nature
ISBN: 3030639630
Category : Science
Languages : en
Pages : 639

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Book Description
This Open Access book gives a comprehensive account of both the history and current achievements of molecular beam research. In 1919, Otto Stern launched the revolutionary molecular beam technique. This technique made it possible to send atoms and molecules with well-defined momentum through vacuum and to measure with high accuracy the deflections they underwent when acted upon by transversal forces. These measurements revealed unforeseen quantum properties of nuclei, atoms, and molecules that became the basis for our current understanding of quantum matter. This volume shows that many key areas of modern physics and chemistry owe their beginnings to the seminal molecular beam work of Otto Stern and his school. Written by internationally recognized experts, the contributions in this volume will help experienced researchers and incoming graduate students alike to keep abreast of current developments in molecular beam research as well as to appreciate the history and evolution of this powerful method and the knowledge it reveals.

Atoms, Solids, and Plasmas in Super-Intense Laser Fields

Atoms, Solids, and Plasmas in Super-Intense Laser Fields PDF Author: Dimitri Batani
Publisher: Springer Science & Business Media
ISBN: 1461513510
Category : Science
Languages : en
Pages : 409

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Book Description
The recent developement of high power lasers, delivering femtosecond pulses of 20 2 intensities up to 10 W/cm , has led to the discovery of new phenomena in laser interactions with matter. At these enormous laser intensities, atoms, and molecules are exposed to extreme conditions and new phenomena occur, such as the very rapid multi photon ionization of atomic systems, the emission by these systems of very high order harmonics of the exciting laser light, the Coulomb explosion of molecules, and the acceleration of electrons close to the velocity of light. These phenomena generate new behaviour of bulk matter in intense laser fields, with great potential for wide ranging applications which include the study of ultra-fast processes, the development of high-frequency lasers, and the investigation of the properties of plasmas and condensed matter under extreme conditions of temperature and pressure. In particular, the concept of the "fast ignitor" approach to inertial confinement fusion (ICF) has been proposed, which is based on the separation of the compression and the ignition phases in laser-driven ICF. The aim of this course on "Atom, Solids and Plasmas in Super-Intense Laser fields" was to bring together senior researchers and students in atomic and molecular physics, laser physics, condensed matter and plasma physics, in order to review recent developments in high-intensity laser-matter interactions. The course was held at the Ettore Majorana International Centre for Scientific Culture in Erice from July 8 to July 14,2000.

Advances in Methods and Applications of Quantum Systems in Chemistry, Physics, and Biology

Advances in Methods and Applications of Quantum Systems in Chemistry, Physics, and Biology PDF Author: Ireneusz Grabowski
Publisher: Springer Nature
ISBN: 3031520785
Category :
Languages : en
Pages : 300

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Book Description


Field Ionization Mass Spectrometry

Field Ionization Mass Spectrometry PDF Author: Hans-D. Beckey
Publisher: Elsevier
ISBN: 1483160114
Category : Science
Languages : en
Pages : 362

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Book Description
Field Ionization Mass Spectrometry focuses on developments in field ionization (FI) mass spectrometry and describes its applications in physical chemistry, with emphasis on mass spectrometric problems. Physico-chemical problems as well as problems of chemical analysis are considered based on issues such as the probability of field ionization; field dissociation and charge distribution; kinetics of ion decomposition in high fields; negative ions; surface diffusion; activation of FI emitters; and elucidation of the structures of organic compounds. This book is comprised of four chapters and begins with a short review on some of the most important directions of research in FI mass spectrometry. Two main fields of research are discussed: physico-chemical investigations and quantitative analysis or structural determination of organic substances. The next chapter is devoted to focusing and non-focusing sources of FI and covers topics such as methods for production of FI tips and thin wires, together with the use of tips and carbon filaments as FI emitters. The last two chapters focus on the application of the FI mass spectrometer to physico-chemical problems and to quantitative analysis of homologous series of organic substances such as alkanes, alkenes, alkynes, amines, and alcohols. This monograph is intended primarily for chemists and mass spectrometrists.

XUV Pump-Probe Experiments on Diatomic Molecules

XUV Pump-Probe Experiments on Diatomic Molecules PDF Author: Kirsten Schnorr
Publisher: Springer
ISBN: 3319121391
Category : Science
Languages : en
Pages : 198

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Book Description
This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy.

Scientific and Technical Aerospace Reports

Scientific and Technical Aerospace Reports PDF Author:
Publisher:
ISBN:
Category : Aeronautics
Languages : en
Pages : 456

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Book Description
Lists citations with abstracts for aerospace related reports obtained from world wide sources and announces documents that have recently been entered into the NASA Scientific and Technical Information Database.

Atoms, Solids, and Plasmas in Super-Intense Laser Fields

Atoms, Solids, and Plasmas in Super-Intense Laser Fields PDF Author: Dimitri Batani
Publisher: Springer Science & Business Media
ISBN: 9780306466151
Category : Science
Languages : en
Pages : 434

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Book Description
Proceedings of the 30th Course of the International School of Quantum Electronics on Atoms, Solids and Plasmas in Super-Intense Laser Fields, held 8-14 July, in Erice, Sicily

Energy Research Abstracts

Energy Research Abstracts PDF Author:
Publisher:
ISBN:
Category : Power resources
Languages : en
Pages : 872

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Book Description