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Author: Martin Bluschke
Publisher: Springer Nature
ISBN: 3030479021
Category : Science
Languages : en
Pages : 170
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Book Description
In this thesis chemical and epitaxial degrees of freedom are used to manipulate charge and spin ordering phenomena in two families of transition metal oxides, while taking advantage of state-of-the-art resonant x-ray scattering (RXS) methods to characterize their microscopic origin in a comprehensive manner. First, the relationship of charge density wave order to both magnetism and the "pseudogap" phenomenon is systematically examined as a function of charge-carrier doping and isovalent chemical substitution in single crystals of a copper oxide high-temperature superconductor. Then, in copper oxide thin films, an unusual three-dimensionally long-range-ordered charge density wave state is discovered, which persists to much higher temperatures than charge-ordered states in other high-temperature superconductors. By combining crystallographic and spectroscopic measurements, the origin of this phenomenon is traced to the epitaxial relationship with the underlying substrate. This discovery opens new perspectives for the investigation of charge order and its influence on the electronic properties of the cuprates. In a separate set of RXS experiments on superlattices with alternating nickel and dysprosium oxides, several temperature- and magnetic-field-induced magnetic phase transitions are discovered. These observations are explained in a model based on transfer of magnetic order and magneto-crystalline anisotropy between the Ni and Dy subsystems, thus establishing a novel model system for the interplay between transition-metal and rare-earth magnetism.
Author: Martin Bluschke
Publisher: Springer Nature
ISBN: 3030479021
Category : Science
Languages : en
Pages : 170
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Book Description
In this thesis chemical and epitaxial degrees of freedom are used to manipulate charge and spin ordering phenomena in two families of transition metal oxides, while taking advantage of state-of-the-art resonant x-ray scattering (RXS) methods to characterize their microscopic origin in a comprehensive manner. First, the relationship of charge density wave order to both magnetism and the "pseudogap" phenomenon is systematically examined as a function of charge-carrier doping and isovalent chemical substitution in single crystals of a copper oxide high-temperature superconductor. Then, in copper oxide thin films, an unusual three-dimensionally long-range-ordered charge density wave state is discovered, which persists to much higher temperatures than charge-ordered states in other high-temperature superconductors. By combining crystallographic and spectroscopic measurements, the origin of this phenomenon is traced to the epitaxial relationship with the underlying substrate. This discovery opens new perspectives for the investigation of charge order and its influence on the electronic properties of the cuprates. In a separate set of RXS experiments on superlattices with alternating nickel and dysprosium oxides, several temperature- and magnetic-field-induced magnetic phase transitions are discovered. These observations are explained in a model based on transfer of magnetic order and magneto-crystalline anisotropy between the Ni and Dy subsystems, thus establishing a novel model system for the interplay between transition-metal and rare-earth magnetism.
Author: Martin Maxmilian Passer Bluschke
Publisher:
ISBN:
Category :
Languages : en
Pages :
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Book Description
Author: A R Bishop
Publisher: World Scientific
ISBN: 981448671X
Category : Science
Languages : en
Pages : 233
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Book Description
There is considerable interest in the intrinsically multiscale structure and dynamics of complex electronic oxides, especially since these materials include those of technological importance, such as colossal magnetoresistance manganites and cuprate high temperature superconductors. Current microscopies, such as diffuse X-ray and inelastic neutron scattering, electromagnetic and acoustic response, NMR and scanning tunneling microscope probes, have revealed static and dynamic multiscale patterns in charge positioning, lattice structure and magnetic orientation, that respond to both external stress and magnetic field. These self-organized patterns include charge and orbital ordering; stripes in strain/spin; and labyrinth-like conductance modulations. The materials exhibit nanoscale phase segregation and mesoscale inhomogeneous clustering, and their phase transitions can have a percolative character.This volume presents experimental and theoretical work on these exciting new developments in condensed matter physics and materials science.
Author:
Publisher:
ISBN:
Category : Chemistry
Languages : en
Pages : 2566
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Book Description
Author: Eva Pavarini
Publisher: Forschungszentrum Jülich
ISBN: 3893368841
Category :
Languages : en
Pages : 562
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Book Description
Author: Janelle Leger
Publisher: CRC Press
ISBN: 1439806896
Category : Science
Languages : en
Pages : 238
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Book Description
With contributions from a community of experts, the book focuses on the use of ionic functions to define the principle of operation in polymer devices. It begins by reviewing the scientific understanding and important scientific discoveries made on the electrochemistry of conjugated polymers. It examines the known effects of ion incorporation, including the theory and modulation of electrochemistry in polymer films, and it explores the coupling of electronic and ionic transport in polymer films.
Author: Claudia Cancellieri
Publisher: Springer
ISBN: 3319749897
Category : Technology & Engineering
Languages : en
Pages : 326
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Book Description
This book summarizes the most recent and compelling experimental results for complex oxide interfaces. The results of this book were obtained with the cutting-edge photoemission technique at highest energy resolution. Due to their fascinating properties for new-generation electronic devices and the challenge of investigating buried regions, the book chiefly focuses on complex oxide interfaces. The crucial feature of exploring buried interfaces is the use of soft X-ray angle-resolved photoemission spectroscopy (ARPES) operating on the energy range of a few hundred eV to increase the photoelectron mean free path, enabling the photons to penetrate through the top layers – in contrast to conventional ultraviolet (UV)-ARPES techniques. The results presented here, achieved by different research groups around the world, are summarized in a clearly structured way and discussed in comparison with other photoemission spectroscopy techniques and other oxide materials. They are complemented and supported by the most recent theoretical calculations as well as results of complementary experimental techniques including electron transport and inelastic resonant X-ray scattering.
Author: Andrei Mourachkine
Publisher: Cambridge Int Science Publishing
ISBN: 1904602274
Category : Technology & Engineering
Languages : en
Pages : 326
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Book Description
Annotation The first book dealing with the subject of room-temperature conductivity.
Author:
Publisher:
ISBN:
Category : Physics
Languages : en
Pages : 1264
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Book Description
Author: Vladislav A. Sadykov
Publisher: Elsevier
ISBN: 012814808X
Category : Technology & Engineering
Languages : en
Pages : 590
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Book Description
Advanced Nanomaterials for Catalysis and Energy: Synthesis, Characterization and Applications outlines new approaches to the synthesis of nanomaterials (synthesis in flow conditions, laser electrodispersion of single metals or alloys on carbon or oxide supports, mechanochemistry, sol-gel routes, etc.) to provide systems with a narrow particle size distribution, controlled metal-support interaction and nanocomposites with uniform spatial distribution of domains of different phases, even in dense sintered materials. Methods for characterization of real structure and surface properties of nanomaterials are discussed, including synchrotron radiation diffraction and X-ray photoelectron spectroscopy studies, neutronography, transmission/scanning electron microscopy with elemental analysis, and more. The book covers the effect of nanosystems' composition, bulk and surface properties, metal-support interaction, particle size and morphology, deposition density, etc. on their functional properties (transport features, catalytic activity and reaction mechanism). Finally, it includes examples of various developed nanostructured solid electrolytes and mixed ionic-electronic conductors as materials in solid oxide fuel cells and asymmetric supported membranes for oxygen and hydrogen separation. - Outlines synthetic and characterization methods for nanocatalysts - Relates nanocatalysts' properties to their specific applications - Proposes optimization methods aiming at specific applications
