Anion Photoelectron Spectroscopy of Metallic Species PDF Download
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Author: Peter William Villalta
Publisher:
ISBN:
Category :
Languages : en
Pages : 560
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Author: Peter William Villalta
Publisher:
ISBN:
Category :
Languages : en
Pages : 560
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Author: Evan Lowell Millam
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Category :
Languages : en
Pages : 280
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Author: Vicki D. Moravec
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Category :
Languages : en
Pages : 502
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Author: Harry Gomez
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Category :
Languages : en
Pages : 482
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Author: David Yubero Valdivielso
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Category :
Languages : en
Pages : 0
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Author: Terry A. Yen
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Category :
Languages : en
Pages : 220
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Abstract Anion Photoelectron Spectroscopy of Exotic Species By Terry A. Yen Doctor of Philosophy in Chemistry University of California, Berkeley Professor Daniel M. Neumark, Chair Anion photoelectron spectroscopy is performed on a variety of small, unstable species in both the gas and condensed phases. For the gas-phase studies, the properties of the astrophysically significant molecules C3N- and C5N- and the biologically meaningful deprotonated DNA nucleobases were investigated. Spectra of C3N- and C5N- were obtained at 283 nm using slow electron velocity-map imaging and at 213 nm using field-free time-of-flight, respectively. Adiabatic electron affinities for both species, a term value for the first excited state of C5N, and vibrational frequencies for the degenerate cis and trans bending modes of C3N were determined. Spectra of deprotonated thymine and deprotonated cytosine at 213 nm were obtained to explore their excited state dynamics to understand the photostability of DNA. For the condensed phase studies, a new spectrometer, the liquid microjet apparatus, was assembled and used to measure the vertical binding energy of the solvated electron. A microjet flowing a salt solution intersects a laser at either 266 nm or 213 nm. Two photons from a single nanosecond laser pulse are used to first generate solvated electrons using charge-transfer-to-solvent excitation and to then eject them into vacuum, where they are detected using field-free time-of-flight.
Author: Stephen R. Miller
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ISBN:
Category :
Languages : en
Pages : 742
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Author: Sean Michael Casey
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Category :
Languages : en
Pages : 520
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Author: Susan Michelle Erickson Green
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Category :
Languages : en
Pages : 390
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Author: Chun-Lin Cheng
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ISBN:
Category :
Languages : en
Pages : 544
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