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Author: Vladimir Lʹvovich Broude
Publisher: Springer
ISBN:
Category : Science
Languages : en
Pages : 296
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Book Description
Author: Vladimir Lʹvovich Broude
Publisher: Springer
ISBN:
Category : Science
Languages : en
Pages : 296
Get Book Here
Book Description
Author: Seogjoo J. Jang
Publisher: Elsevier
ISBN: 0081023359
Category : Science
Languages : en
Pages : 242
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Book Description
Dynamics of Molecular Excitons provides a comprehensive, but concise description of major theories on the dynamics of molecular excitons, intended to serve as a self-contained resource on the topic. Designed to help those new to this area gain proficiency in this field, experts will also find the book useful in developing a deeper understanding of the subject. The starting point of the book is the standard microscopic definition of molecular Hamiltonians presented in commonly accepted modern quantum mechanical notations. Major assumptions and approximations involved in constructing Frenkel-type exciton Hamiltonians, which are well established, but are often hidden under arcane notations and approximations of old publications, are presented in detail. This will help quantum chemists understand the major assumptions involved in the definition of commonly used exciton models. Rate theories of exciton dynamics, such as Förster and Dexter theories and their modern generalizations, are presented in a unified and detailed manner. In addition, important aspects that are often neglected, such as local field effect and the role of fluctuating environments, are discussed. Various quantum dynamics methods allowing coherent dynamics of excitons are presented in a systematic manner in the context of quantum master equations or path integral formalisms. The author also provides a detailed theoretical explanation for the major spectroscopic techniques probing exciton dynamics, including modern two-dimensional electronic spectroscopy, with a critical assessment of the implications of these spectroscopic measurements. Finally, the book includes a brief overview of major applications including an explanation of organic photovoltaic materials and natural light harvesting complexes.
Author: Seogjoo J. Jang
Publisher: Elsevier
ISBN: 0081023367
Category : Science
Languages : en
Pages : 244
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Book Description
Dynamics of Molecular Excitons provides a comprehensive, but concise description of major theories on the dynamics of molecular excitons, intended to serve as a self-contained resource on the topic. Designed to help those new to this area gain proficiency in this field, experts will also find the book useful in developing a deeper understanding of the subject. The starting point of the book is the standard microscopic definition of molecular Hamiltonians presented in commonly accepted modern quantum mechanical notations. Major assumptions and approximations involved in constructing Frenkel-type exciton Hamiltonians, which are well established, but are often hidden under arcane notations and approximations of old publications, are presented in detail. This will help quantum chemists understand the major assumptions involved in the definition of commonly used exciton models. Rate theories of exciton dynamics, such as Förster and Dexter theories and their modern generalizations, are presented in a unified and detailed manner. In addition, important aspects that are often neglected, such as local field effect and the role of fluctuating environments, are discussed. Various quantum dynamics methods allowing coherent dynamics of excitons are presented in a systematic manner in the context of quantum master equations or path integral formalisms. The author also provides a detailed theoretical explanation for the major spectroscopic techniques probing exciton dynamics, including modern two-dimensional electronic spectroscopy, with a critical assessment of the implications of these spectroscopic measurements. Finally, the book includes a brief overview of major applications including an explanation of organic photovoltaic materials and natural light harvesting complexes. - Covers major theories of exciton dynamics in a consciously concise and easily readable way - Bridges the gap between quantum dynamics working with phenomenological exciton Hamiltonian and quantum chemistry construct reliable models amenable for dynamics calculations from ab initio calculations - Explores modern nonlinear electronic spectroscopy techniques to probe exciton dynamics, showing how it is applied
Author: Herbert van Amerongen
Publisher: World Scientific
ISBN: 9789810232801
Category : Science
Languages : en
Pages : 612
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Book Description
Excitons are considered as the basic concept used by describing the spectral properties of photosynthetic pigment-protein complexes and excitation dynamics in photosynthetic light-harvesting antenna and reaction centers. Following the recently obtained structures of a variety of photosynthetic pigment-protein complexes from plants and bacteria our interest in understanding the relation between structure, function and spectroscopy has strongly increased. These data demonstrate a short interpigment distance (of the order of 1 nm or even smaller) and/or a highly symmetric (ring-like) arrangement of pigment molecules in peripheral light-harvesting complexes of photosynthetic bacteria. Books which were devoted to the exciton problem so far mainly considered the spectral properties of molecular crystals. However, the small size of these pigment aggregates in the pigment-protein complexes as well as the role of the protein, which is responsible for the structural arrangement of the complex, clearly will have a dramatic influence on the pigment spectra and exciton dynamics. All these aspects of the problem are considered in this book. Exciton theory is mainly considered for small molecular aggregates (dimers, ring-like structures etc.). Together with the theoretical description of the classical conceptual approach, which mainly deals with polarization properties of the absorption and fluorescence spectra, the nonlinear femtosecond spectroscopy which is widely used for investigations now is also discussed. A large part of the book demonstrates the excitonic effects in a multitude of photosynthetic pigment-protein complexes and how we can understand these properties on the basis of the exciton concept.
Author: O. Sild
Publisher: Elsevier
ISBN: 1483284751
Category : Science
Languages : en
Pages : 255
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Book Description
Molecular Spectroscopy–XI provides information pertinent to the fundamental aspects of molecular spectroscopy. This book discusses the modifications of molecular spectra when the density varies as a function of temperature and pressure. Organized into 15 chapters, this book begins with an overview of the several processes concerning triplet excitons leading to magnetic-field sensitive luminescence in organic crystals and related compounds. This text then examines the methods of investigation of the exciton band structures in molecular crystals. Other chapters consider the conditions for the equivalence of Fourier spectroscopy and of slow passage experiments in nuclear magnetic resonance. This book discusses as well the application of computer technology in carbon-13 magnetic resonance spectroscopy. The final chapter deals with the application of high-resolution proton and carbon-13 n.m.r. spectroscopy for the investigation of the molecular conformations in proteins. This book is a valuable resource for organic chemists, biologists, microbiologists, scientists, and research workers.
Author: Vladimir L. Broude
Publisher: Springer
ISBN: 9783642882203
Category : Science
Languages : en
Pages : 0
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Book Description
Low-temperature spectroscopy of organic molecular crystals came into being in the late 20s, just when quantum physics of solids as a whole began to de velop vigorously. Already in the early works, two experimental facts of prime importance were discovered: the presence of a multitude of narrow bands in the low-temperature spectrum of a crystal, and a close relationship between the spectrum of the crystal and that of the constituent molecules. These findings immediately preceded the celebrated paper of Frenkel in which he went beyond the framework of Bloch's scheme and advanced the exciton concept. Subsequent investigations showed that the most interesting features of the spectra of molecular crystals are associated with excitons, and then the spectroscopy of molecular excitons began to form gradually on the basis of the spectroscopy of organic crystals. The molecular exciton became synonymous to the Frenkel exciton in a molecular crystal. In view of the difficulties involved in the analysis of rich spectra con taining many tens of bands, the spectroscopy of molecular crystals had long been connected most closely with the spectroscopy of molecules. It had deve loped independently, to a large extent, from the other branches of solid state physics. This was also emphasized by the difference in experimental techniques, the specific properties of the objects, etc. As a result, there was some lag in ideas and concepts.
Author: Leonas Valkunas
Publisher: John Wiley & Sons
ISBN: 3527653678
Category : Science
Languages : en
Pages : 414
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Book Description
This work brings together quantum theory and spectroscopy to convey excitation processes to advanced students and specialists wishing to conduct research and understand the entire fi eld rather than just single aspects. Written by experienced authors and recognized authorities in the field, this text covers numerous applications and offers examples taken from different disciplines. As a result, spectroscopists, molecular physicists, physical chemists, and biophysicists will all fi nd this a must-have for their research. Also suitable as supplementary reading in graduate level courses.
Author: A. Davydov
Publisher: Springer
ISBN: 1489951695
Category : Science
Languages : en
Pages : 319
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Book Description
Author: Baldassare Di Bartolo
Publisher: Springer Science & Business Media
ISBN: 1468427938
Category : Science
Languages : en
Pages : 423
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Book Description
These proceedings report the lectures and seminars presented at the NATO Advanced Study Institute on "The Spectroscopy of the Excited State," held at Erice, Italy, June 9-24, 1975. This Institute was an activity of the International School of Atomic and Molecular Spectroscopy of the "Ettore Majorana" Centre for Scientific Culture. The Institute consisted of a series of lectures on the spectroscopic properties of materials in excited electronic states, that, starting at a fundamental level, finally reached the current level of research. The sequence of lectures and the organization of the material taught were in keeping with a didac tical presentation. In essence the course had the two-fold pur pose of organizing what was known on the subject, and updating the knowledge in the field. The formal lectures were complemented by seminars whose abstracts are also included in these proceedings. The proceedings report also the contributions sent by Professors R.G.W. Norrish and S. C1aesson who, unfortunately, were not able to come because of illness. A total of 62 participants and 7 lecturers came from the following countries: Belgium, Canada, Czechoslovakia, France, Germany, Israel, Italy, Japan, Netherlands, Norway, Pakistan, Poland, Sweden, Switzerland, the United Kingdom, the United States and Venezuela. The secretaries of the course were: A. La Francesca for the administrative aspects of the meeting and P.Papagiannakopou10s for the scientific aspects of the meeting.
Author: Vladimir L. Broude
Publisher: Springer
ISBN: 9783540124092
Category : Technology & Engineering
Languages : en
Pages : 274
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Book Description
Low-temperature spectroscopy of organic molecular crystals came into being in the late 20s, just when quantum physics of solids as a whole began to de velop vigorously. Already in the early works, two experimental facts of prime importance were discovered: the presence of a multitude of narrow bands in the low-temperature spectrum of a crystal, and a close relationship between the spectrum of the crystal and that of the constituent molecules. These findings immediately preceded the celebrated paper of Frenkel in which he went beyond the framework of Bloch's scheme and advanced the exciton concept. Subsequent investigations showed that the most interesting features of the spectra of molecular crystals are associated with excitons, and then the spectroscopy of molecular excitons began to form gradually on the basis of the spectroscopy of organic crystals. The molecular exciton became synonymous to the Frenkel exciton in a molecular crystal. In view of the difficulties involved in the analysis of rich spectra con taining many tens of bands, the spectroscopy of molecular crystals had long been connected most closely with the spectroscopy of molecules. It had deve loped independently, to a large extent, from the other branches of solid state physics. This was also emphasized by the difference in experimental techniques, the specific properties of the objects, etc. As a result, there was some lag in ideas and concepts.
