Author: Robin P. Gardner
Publisher:
ISBN:
Category :
Languages : en
Pages :

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This research project was to improve the prompt gamma-ray neutron activation analysis (PGNAA) measurement approach for bulk analysis, oil well logging, and small sample thermal enutron bean applications.

Author: G. Molnar
Publisher: Springer Science & Business Media
ISBN: 0387233598
Category : Science
Languages : en
Pages : 448

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Book Description
Prompt gamma activation analysis (PGAA) is a unique, non-destructive nuclear analytical method with multi-element capabilities. It is most effective if intense neutron beams (especially cold beams) of nuclear reactors are used to induce the prompt gamma radiation. Based largely on the authors' pioneering research in cold neutron PGAA, the handbook describes the methodology in self-contained manner and reviews recent applications. The library of prompt gamma ray data and spectra for all natural elements is a unique aid to the practitioner. The level is understandable by a broad audience, which facilitates teaching and training. The Handbook of Prompt Gamma Activation Analysis is a comprehensive handbook written for those practising the method, wanting to implement it at a reactor facility, or just looking for a powerful non-destructive method of element analysis. The book is also useful for nuclear physics, chemistry and engineering scientists, scholars and graduate students interested in neutron-induced gamma ray spectroscopy and nuclear analytical methods.

Author: Abdul-Salam Gubreal Hanna
Publisher:
ISBN:
Category :
Languages : en
Pages : 342

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Author:
Publisher:
ISBN:
Category :
Languages : en
Pages :

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Prompt Gamma-Ray Neutron Activation Analysis (PGNAA) offers a non-destructive, relatively rapid on-line method for determination of elemental composition of bulk and other samples. However, PGNAA has an inherently large background. These backgrounds are primarily due to the presence of the neutron excitation source. It also includes neutron activation of the detector and the prompt gamma rays from the structure materials of PGNAA devices. These large backgrounds limit the sensitivity and accuracy of PGNAA. Since Most of the prompt gamma rays from the same element are emitted in coincidence, a possible approach for further improvement is to change the traditional PGNAA detection technique and introduce the gamma-gamma coincidence technique. It is well known that the coincidence technique can eliminate most of the interference backgrounds and improve the signal-to-noise ratio. A new Monte Carlo code CEARCPG is being developed at CEAR to predict coincidence counting in coincidence PGNAA. Compared to the other existing Monte Carlo code, a new algorithm of sampling the prompt gamma rays, which are produced from neutron capture reaction and neutron inelastic scattering reaction, is developed in this work. All the prompt gamma rays are taken into account by using this new algorithm. Before this work, the commonly used method is to interpolate the prompt gamma rays from the pre-calculated gamma-ray table. It works fine for the single spectrum. However it limits the capability to simulate the coincidence spectrum. This new algorithm is to sample the prompt gamma rays from the nucleus scheme. It makes possible to simulate the coincidence spectrum by using Monte Carlo method. The primary nuclear data library used to sample the prompt gamma rays comes from ENSDF library. Three cases are simulated and the simulated results are checked with the experiments. The first case is the prototype for ETI PGNAA application. This case is designed to check the capability of CEARCPG for sing.

Author: International Atomic Energy Agency
Publisher: IAEA
ISBN:
Category : Science
Languages : en
Pages : 282

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Book Description
Neutron-capture prompt-gamma activation analysis (PGAA) is particularly valuable as a non-destructive nuclear method in the measurement of elements that do not form neutron capture products with delayed gamma ray emissions. Inaccurate and incomplete data have been a significant hindrance in the qualitative and quantitative analysis of complicated capture gamma spectra by means of PGAA. This database was produced to improve the quality and quantity of required data in order to make possible the reliable application of PGAA in fields such as materials science, geology, mining, archaeology, environment, food analysis and medicine. The database provides a variety of tables for all natural elements (from H to U) including the following data: isotopic composition, thermal radiative cross-section (total and partial), Westcott g-factors, energy of the gamma rays (prompt and delayed), decay mode, half-life and branching ratios. The CD-ROM included in this publication contains the database, the retrieval system and important electronic documents related to the project.--Publisher's description.

Author: Joshua A. Robinson
Publisher:
ISBN:
Category : Nuclear activation analysis
Languages : en
Pages : 260

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Book Description
In this work a prompt gamma neutron activation analysis (PGNAA) facility has been designed, built, and characterized at the Oregon State University TRIGA® reactor. PGNAA is a technique used to determine the presence and quantity of trace elements such as boron, hydrogen and carbon which are more difficult to detect with other neutron analysis methods. In PGNAA, isotopes are subjected to a neutron beam, resulting in the formation of an unstable compound nucleus. The compound nucleus immediately decays, producing a series of gamma-rays, whose energies are distinctive to each element. These gamma-rays are then measured using an HPGe detector to determine the elemental composition of the sample. The measured thermal and epithermal neutron fluxes of the PGNAA facility at Oregon State University are 2.81 x 107 ± 5.13 x 105 cm−2s−1 and 1.70 x 104 ± 3.11 x 102 cm−2s−1 respectively. This gives the facility a cadmium ratio of 106. Measured detection limits for boron, chlorine, and potassium in SRM 1571 orchard leaf standard were, 5.6 x 10−4mg/g, 8.2 x 10−2 mg/g and, 1.0 mg/g respectively. Also, the detection limit for hydrogen in high-density polyethylene is, 6.8 x 10−2mg/g. Detection limits for additional elements are presented in this work.

Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 5

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The normal prompt gamma-ray neutron activation analysis for either bulk or small beam samples inherently has a small signal-to-noise (S/N) ratio due primarily to the neutron source being present while the sample signal is being obtained. Coincidence counting offers the possibility of greatly reducing or eliminating the noise generated by the neutron source. The present report presents our results to date on implementing the coincidence counting PGNAA approach. We conclude that coincidence PGNAA yields: (1) a larger signal-to-noise (S/N) ratio, (2) more information (and therefore better accuracy) from essentially the same experiment when sophisticated coincidence electronics are used that can yield singles and coincidences simultaneously, and (3) a reduced (one or two orders of magnitude) signal from essentially the same experiment. In future work we will concentrate on: (1) modifying the existing CEARPGS Monte Carlo code to incorporate coincidence counting, (2) obtaining coincidence schemes for 18 or 20 of the common elements in coal and cement, and (3) optimizing the design of a PGNAA coincidence system for the bulk analysis of coal.

Author: H. D. Choi
Publisher:
ISBN:
Category :
Languages : en
Pages :

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Book Description
The increasing importance of Prompt Gamma-ray ActivationAnalysis (PGAA) in a broad range of applications is evident, and has beenemphasized at many meetings related to this topic (e.g., TechnicalConsultants' Meeting, Use of neutron beams for low- andmedium-fluxresearch reactors: radiography and materialscharacterizations, IAEA Vienna, 4-7 May 1993, IAEA-TECDOC-837, 1993). Furthermore, an Advisory Group Meeting (AGM) for the Coordination of theNuclear Structure and Decay Data Evaluators Network has stated that thereis a need for a complete and consistent library of cold- and thermalneutron capture gammaray and cross-section data (AGM held at Budapest,14-18 October 1996, INDC(NDS)-363); this AGM also recommended theorganization of an IAEA CRP on the subject. The International NuclearData Committee (INDC) is the primary advisory body to the IAEA NuclearData Section on their nuclear data programmes. At a biennial meeting in1997, the INDC strongly recommended that the Nuclear Data Section supportnew measurements andupdate the database on Neutron-induced PromptGamma-ray Activation Analysis (21st INDC meeting, INDC/P(97)-20). As aconsequence of the various recommendations, a CRP on "Development of aDatabase for Prompt Gamma-ray Neutron Activation Analysis (PGAA)" wasinitiated in 1999. Prior to this project, several consultants had definedthe scope, objectives and tasks, as approved subsequently by the IAEA. Each CRP participant assumed responsibility for the execution of specifictasks. The results of their and other research work were discussed andapproved by the participants in research co-ordination meetings (seeSummary reports: INDC(NDS)-411, 2000; INDC(NDS)-424, 2001; andINDC(NDS)-443, 200). PGAA is a non-destructive radioanalytical method, capable of rapid or simultaneous "in-situ" multi-element analyses acrossthe entire Periodic Table, from hydrogen to uranium. However, inaccurateand incomplete data were a significant hindrance in the qualitative andquantitative analysis of complicated capture-gamma spectra by means ofPGAA. Therefore, the main goal of the CRP was to improve the quality andquantity of the required data in order to make possible the reliableapplication of PGAA in fields such as materials science, chemistry, geology, mining, archaeology, environment, food analysis and medicine. This aim wasachieved thanks to the dedicated work and effort of theparticipants. The CD-ROM included with this publication contains thedatabase, the retrieval system, the three CRM reports, and otherimportant electronic documents related to the CRP. The IAEA wishes tothanks all CRP participants who contributed to the success of the CRP and the formulation of this publication. Special thanks are due to R.B. Firestone for his leading roll in the development of this CRP and hiscomprehensive compilation, analysis and provision of the adopteddatabase, and to V. Zerkin for the software developments associatedwiththe retrieval system. An essential component of this data compilation isthe extensive sets of new measurements of capture gamma-ray energies andintensities undertaken at Budapest by Zs. Revay under the direction ofG. L. Molnar. The extensive participation and assistance of H.D. Choi isalso greatly appreciated. Other participants inthis CRP were: R.M. Lindstrom, S.M. Mughabghab, A.V.R. Reddy, V.H. Tan and C.M. Zhou. Thanksare also due to S.C. Frankle and M.A. Lone for their active participationas consultants at some of the meetings. Finally, the participants wish tothank R. Paviotti-Corcuera (Nuclear Data Section, Division of Physicaland Chemical Sciences), who was the IAEA responsible officer for the CRP, this publication and the resulting database. The participants aregrateful to D.L. Muir and A.L. Nichols, successive Heads of the NuclearData Section, for their active and enthusiastic encouragement infurthering the work of the CRP.

Author: Zeev B. Alfassi
Publisher: CRC PressI Llc
ISBN: 9780849351495
Category : Science
Languages : en
Pages : 244

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Book Description
Prompt Gamma Neutron Activation Analysis introduces the fundamental principals and the unique characteristics of the gamma-ray activation method together with its applications and limitations. Sample preparation, instruments, shielding and irradiation using prompt gamma-ray activation analysis techniques with various neutron sources are described in detail. The neutron damage to PGAA instruments, particularly the radiation detector, is investigated. The book compares unique features and limitations of PGAA versus conventional NAA methods. Approximately 50 tables help to illustrate and describe these exciting new methods.

Author: Michael Spychala
Publisher:
ISBN:
Category :
Languages : en
Pages : 9

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Book Description