Microbial and Photochemical Degradation of Allochthonous Dissolved Organic Matter Within River Systems and Watersheds PDF Download
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Author: Tracy Nicole Wiegner
Publisher:
ISBN:
Category :
Languages : en
Pages : 450
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Book Description
Author: Tracy Nicole Wiegner
Publisher:
ISBN:
Category :
Languages : en
Pages : 450
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Book Description
Author: Rainer Maria Wolfgang Amon
Publisher:
ISBN:
Category : Aquatic ecology
Languages : en
Pages : 0
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Book Description
Author: Paula G. Coble
Publisher: Cambridge University Press
ISBN: 0521764610
Category : Science
Languages : en
Pages : 407
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Book Description
A core text on principles, laboratory/field methodologies, and data interpretation for fluorescence applications in aquatic science, for advanced students and researchers.
Author:
Publisher:
ISBN:
Category : Dissertations, Academic
Languages : en
Pages : 756
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Book Description
Author: Stuart Findlay
Publisher: Academic Press
ISBN: 0122563719
Category : Nature
Languages : en
Pages : 534
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Book Description
Overviews of the source, supply and variability of DOM, surveys of the processes that mediate inputs to microbial food webs, and syntheses consolidating research findings provide a comprehensive review of what is known of DOM in freshwater. This book will be important to anyone interested in understanding the fundamental factors associated with DOM that control aquatic ecosystems."--BOOK JACKET.
Author: Ryan H. S. Hutchins
Publisher:
ISBN:
Category :
Languages : en
Pages : 99
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Book Description
Dissolved organic carbon (DOM) is one of the largest cycled organic carbon pools on Earth and an important biogeochemical factor in aquatic systems. DOM can act as an energy source for microorganisms, alter the depth of the photic zone for photosynthesis, absorb harmful ultraviolet radiation, as well as alter the transport and toxicity of contaminants. The purpose of this research project was to characterize DOM in the Grand River watershed in Ontario, Canada using a wide range of qualitative and quantitative techniques and determine the impact of anthropogenic activities as well as seasonal and longitudinal changes on DOM processes. To reach the study objectives, historical data was analyzed to determine the seasonal cycle in the Grand River watershed. Intensive longitudinal sampling surveys were undertaken to evaluate the DOM characteristics and processes in the Grand River. Surveys of the less impacted Burnt River watershed were used as a comparison watershed to the Grand River to evaluate allochthonous and autochthonous indicators of DOM source and human impacts on DOM processes. Drinking water surveillance data was used to evaluate the effect of DOM in the Grand River on formation of disinfection by-products (DBPs). Different trends were seen in the Grand River in terms of longitudinal area and season. The headwaters of the river showed more autochthonous DOM in the spring and winter compared to the fall and summer. The lower-central river peaked in autochthonous DOM in the summer and was more allochthonous in the winter. DOM generally became more autochthonous downstream in the Grand River and was most autochthonous below the large sewage treatment plants (STPs) in the central portion. Protein content, measured as protein-like fluorescence normalized to DOC concentration, was strongly related to [delta]15N of DON; both are associated with autochthonous DOM in the Grand River and show the effects of the major STPs. The increase in autochthonous DOM below the STPs is likely associated with nutrient enrichment stimulating primary production and macrophyte growth. Based on the comparison of the Burnt River with the more impacted Grand River, the effect of lakes and photodegradation can make discrimination of autochthonous and allochthonous DOM more difficult. The ratio of DOC/DON and protein-like fluorescence proved to be robust indicators despite photodegradation. Human impacts on the Grand River watershed result in a greater seasonal cycle, high primary production in the summer and a downstream trend of increasing autochthonous DOM compared to the Burnt River. Based on drinking water surveillance data and literature review, autochthonous DOM caused greater DBPs in the drinking waters fed by the Grand River. This is currently a threat to human health and DBPs in sewage treatment plant effluent may be a threat to ecosystem health.
Author: Khan M.G. Mostofa
Publisher: Springer Science & Business Media
ISBN: 3642322239
Category : Science
Languages : en
Pages : 919
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Book Description
Photoinduced processes, caused by natural sunlight, are key functions for sustaining all living organisms through production and transformation of organic matter (OM) in the biosphere. Production of hydrogen peroxide (H2O2) from OM is a primary step of photoinduced processes, because H2O2 acts as strong reductant and oxidant. It is potentially important in many aquatic reactions, also in association with photosynthesis. Allochthonous and autochthonous dissolved organic matter (DOM) can be involved into several photoinduced or biological processes. DOM subsequently undergoes several physical, chemical, photoinduced and biological processes, which can be affected by global warming. This book is uniquely structured to overview some vital issues, such as: DOM; H2O2 and ROOH; HO•; Degradation of DOM; CDOM, FDOM; Photosynthesis; Chlorophyll; Metal complexation, and Global warming, as well as their mutual interrelationships, based on updated scientific results.
Author: Xiaping Li
Publisher:
ISBN:
Category : Electronic dissertations
Languages : en
Pages : 73
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Book Description
The objective of the present study was to provide better understanding of the effects of watershed land use on molecular composition of streamwater DOM and molecular transformations associated with photochemical and microbial processing of DOM. We compared DOM from headwater streams draining forest-dominated watersheds (FW) and pasture-dominated watersheds (PW) in the lower Chesapeake Bay region (Virginia, USA). Electrospray Ionization Fourier Transform Ion Cyclotron Resonance Mass Spectrometry analysis was conducted on streamwater DOM prior to and after laboratory incubations: 1) bacteria-only incubations; 2) light-only incubations; and 3) combined light+bacterial incubations. Results showed that DOM in FW streams and PW streams differed in molecular characteristics--the former was characterized by greater structural complexity and aromaticity, higher proportions of condensed aromatic molecules and black carbon-like components, while the latter was higher in the proportions of lipid-like components, protein-like components and aliphatic compounds. Relative to DOM from FW streams, DOM from PW streams was more reactive to bacterial transformation. Protein-like components, lipid-like components and unsaturated hydrocarbon-like components are primarily responsible for the changes associated with bacterial transformation of DOM. However, similar behavior was also observed for DOM in FW streams and PW streams under the influence of bacterial and photochemical processes. Bacterial transformation reduced the proportions of lipid-like components but increased the proportions of lignin-like components and carboxyl-rich alicyclic molecule-like components, indicating that lipid-like components was a bioreactive class while lignin-like components and carboxyl-rich alicyclic were resistant to bacterial processing. Photochemical processes, alone or combined with microbial alterations, increased the proportions of protein-like components, which may be due to the light stimulation of autochthonous production of protein-like components, and increased the relative abundance of carboxyl-rich alicyclic molecule-like components, which indicates the refractory nature of these molecules. Photochemical processes also significantly reduced the amount of dissolved black carbon-like components, which suggests dissolved black carbon was a photoreactive class, countering the conventional view that black carbon was an inter group in carbon cycle. Collectively, these findings suggest that human land use in upstream watersheds may lead to alterations to the molecular composition of streamwater DOM as well as to its behavior to photochemical and microbial processing.
Author: Peter Brimblecombe
Publisher: Springer Science & Business Media
ISBN: 1402058853
Category : Science
Languages : en
Pages : 405
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Book Description
This book looks at the sources and composition of the atmosphere and rainfall, with particular attention on acidifying components and those that affect ecosystems. It further widens the subject to look at trace metals. It includes papers on the impact of deposition on soils and forests and the recovery of the natural environment. Work on critical loads makes a contribution to understanding the degree to which deposition must be reduced to limit its impact.
Author: Rachel Elizabeth Sipler
Publisher:
ISBN:
Category : Aquatic ecology
Languages : en
Pages : 179
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Book Description
Dissolved organic matter (DOM) is an important source of nutrients in aquatic systems contributing to the growth of phytoplankton and bacteria. The overall response appears to be driven by the phytoplankton and bacteria species present as well as the composition of DOM provided. This dissertation explores the bioavailability of allochthonous and autochthonous DOM sources to, and its affect on, the growth of marine phytoplankton and bacterial community abundance and composition. This research utilizes advanced chemical (electrospray ionization mass spectrometry (ESI-MS)) and molecular (terminal restriction fragment length polymorphism (TRFLP)) techniques to characterize the DOM and microbial community. To investigate the role of allochthonous DOM in phytoplankton growth, DOM from two different riverine sources from watersheds with different land use practices, was supplied to a natural cyanobacteria population. The bioavailability of autochthonous DOM was investigated by supplying DOM produced by a single culture of cyanobacteria to a natural dinoflagellate bloom community. The potential negative effect of an individual autochthonous DOM compound was investigated through the addition of marine toxin, brevetoxin, to three different natural bacterial communities. This dissertation resulted in the first ESI-MS characterization spectra of the DOM associated with three different natural phytoplankton blooms, a culture of cyanobacteria, and two different South Florida rivers. It was also the first study to identify previously uncharacterized allochthonous and autochthonous DOM masses bioavailable to natural marine phytoplankton communities. Bulk level analyses within these experiments quantified lower limits for the bioavailability of allochthonous and autochthonous DOM sources and the relative community response to each of these sources. This dissertation also represents the first molecular evaluation of the bacteria associated with a bloom and the first investigation of the allelopathic properties of brevetoxin. It has discussed and applied the use of ESI-MS to investigate the bioavailability of complex DOM, identified and quantified potential nutrient sources and linked marine toxin production to changes in bacterial community composition.
