Few Recent Experiments on Surface Studies by Second Harmonic Generation PDF Download
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Languages : en
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Surface second harmonic generation (SHG) is used to monitor adsorption and desorption of molecules on metal and semiconductor surfaces in ultrahigh vacuum. Surface SHG has also been used to study monolayers of molecules at a liquid/air interface. 13 refs., 6 figs. (WRF).
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Languages : en
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Surface second harmonic generation (SHG) is used to monitor adsorption and desorption of molecules on metal and semiconductor surfaces in ultrahigh vacuum. Surface SHG has also been used to study monolayers of molecules at a liquid/air interface. 13 refs., 6 figs. (WRF).
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Languages : en
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Optical second-harmonic generation (SHG) is sensitive enough to respond to a submonolayer of surface atoms or molecules. It can therefore be used to probe surfaces or interfaces between two centrosymmetric media. The surface-specific nature of this optical method offers some advantages. We have demonstrated in recent experiments that resonant SHG can allow us to obtain spectroscopic data of submonolayers of adsorbed molecules on a surface. The signal was so strong that less than one tenth of a monolayer of dye molecules could be easily detected. The method can be applied to molecules adsorbed at an interface between two dense media such as a liquid/solid interface. Then, using SHG, adsorption isotherms of adsorbates on substrates can be measured. One is often interested in how large the bulk contribution to SHG is in comparison with the surface contribution. Second-order nonlinear optical processes are forbidden in a medium with inversion symmetry only in the electric-dipole approximation. Could SGH from electric-quadrupole and magnetic-dipole contributions in the bulk be so strong as to mask out the electric-dipole contribution from the surface. We have found that the SH signal from a centrosymmetric substrate can be changed appreciably by the adsorption of a monolayer. This clearly indicates that it is the adsorbate layer rather than the bulk of the substrate which dominates the SHG process. We are, however, also interested in developing the SHG technique for studying bare surfaces, and would like to know the relative bulk and surface contribution to SHG in such cases. We have studied this problem experimentally by measuring the SHG from well-defined faces of a crystalline material.
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Category : Power resources
Languages : en
Pages : 464
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Author: Pierre-François Brevet
Publisher: EPFL Press
ISBN: 9782880743451
Category : Electrochemistry
Languages : en
Pages : 162
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Author: Gabriella Cerrone
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Category :
Languages : en
Pages : 0
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Author: F.R. Aussenegg
Publisher: Springer Science & Business Media
ISBN: 3642820859
Category : Science
Languages : en
Pages : 250
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The physics and chemistry of surfaces is becoming more and more important as an exciting field of basic research as well as in devices and technology. The diagnoses and the conditioning of surfaces and studies of molecular interac tions with surfaces have made large advancements by using laser techniques. With its divisional meeting 1983 the Quantum Electronics Division of the European Physical Society tried to set up a forum where the latest ideas and achievements could be presented and discussed. The wide range of topics (gen eral surface spectroscopy, surface-enhanced optical processes, laser surface spectroscopy, laser-induced processes at surfaces) was deliberately chosen to provide an opportunity for specialists from one field to get acquainted with the techniques and results from others. This meeting took place in Mauterndorf, Austria, from March 9th to March 11th, 1983. Mauterndorf is a small village in the Austrian Alps, situated in a well-known skiing area. The conference was held in a medieval castle adapt ed as a conference center. These stimulating surroundings guaranteed a vivid exchange of ideas among the 98 participants from 17 nations. Among the numerous people engaged in the organization, our special thanks go to Mrs. I. Mandl and Mrs. B. Seeberg for doing a superb job in implementing the meeting arrangements and efficiently prompting the authors to deliver their manuscripts for this volume in time.
Author: Francesco S. Pavone
Publisher: Taylor & Francis
ISBN: 1439849153
Category : Science
Languages : en
Pages : 465
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Second-harmonic generation (SHG) microscopy has shown great promise for imaging live cells and tissues, with applications in basic science, medical research, and tissue engineering. Second Harmonic Generation Imaging offers a complete guide to this optical modality, from basic principles, instrumentation, methods, and image analysis to biomedical a
Author: Yehiam Prior
Publisher: Springer Science & Business Media
ISBN: 1461594596
Category : Science
Languages : en
Pages : 482
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The Fritz Haber Symposium on Methods of Laser Spectroscopy was held in Ein Bokek, Israel, on the shores of the Dead Sea, on December 16-20, 1985. The location is the lowest place on earth, 392 meters below sea level. It was hoped that 120 active laser scientists, so lowly trapped in such a place, with the nearest entertainment 100 km away, will have no choice but to discuss laser spectroscopy. On the average, the Dead Sea area receives 3-4 days of rain each year, and this year these days all occurred during the conference. This did not mean the cancellation of the hikes, although the trip to Massada was conducted in the rain. The unexpected rains also caused flash floods in the area, and Ein Bokek was completely cut-off on Thursday night. The archeologist scheduled to speak after dinner, and the belly dancer scheduled to appear afterwards, (~ould not arrive, resulting in the only serious deviation from the original plan. The scientific program consisted of invited talks and contributed posters. The emphasis in selection of invited speakers and topics was on the methods rather than specific molecular systems, and an attempt was made to allow ample time for discussion after each lecture. The same philosophy guided us in editing this book, and authors were requested to write manuscripts longer than usual for standard conference proceedings.
Author: Arthur T. Hubbard
Publisher: CRC Press
ISBN: 100071490X
Category : Computers
Languages : en
Pages : 928
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This exciting new handbook investigates the characterization of surfaces. It emphasizes experimental techniques for imaging of solid surfaces and theoretical strategies for visualization of surfaces, areas in which rapid progress is currently being made. This comprehensive, unique volume is the ideal reference for researchers needing quick access to the latest developments in the field and an excellent introduction to students who want to acquaint themselves with the behavior of electrons, atoms, molecules, and thin-films at surfaces. It's all here, under one cover! The Handbook of Surface Imaging and Visualization is filled with sixty-four of the most powerful techniques for characterization of surfaces and interfaces in the material sciences, medicine, biology, geology, chemistry, and physics. Each discussion is easy to understand, succinct, yet incredibly informative. Data illustrate present research in each area of study. A wide variety of the latest experimental and theoretical approaches are included with both practical and fundamental objectives in mind. Key references are included for the reader's convenience for locating the most recent and useful work on each topic. Readers are encouraged to contact the authors or consult the references for additional information. This is the best ready reference available today. It is a perfect source book or supplemental text on the subject.
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Category : Physics
Languages : en
Pages : 1416
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